Suggestions by @jahzeelperez

Curtis Armstrong

as Game Master in The Smurfs (Animated Series)

Richard Kind

as Dr. Charlatan in The Smurfs (Animated Series)

Adam DeVine

as No Name Smurf in The Smurfs (Animated Series)

Quinton Flynn

as Archer Smurf in The Smurfs (Animated Series)

Josh Gad

as Scaredy Smurf in Making a good Smurfs movie reboot

Maile Flanagan

as Scruple in The Smurfs (Animated Series)

Ed Helms

as Farmer Smurf in Making a good Smurfs movie reboot

Kieran Culkin

as Brainy Smurf in The Smurfs (Animated Series)

Eric Bauza

as Party-Planner Smurf in The Smurfs (Animated Series)

Paul F. Tompkins

as Reporter Smurf in The Smurfs (Animated Series)

Glenn Close

as Nanny Smurf in The Smurfs (Animated Series)

Carol Kane

as Bignose in The Smurfs (Animated Series)

Kari Wahlgren

as Lydia in The Smurfs (Animated Series)

John DiMaggio

as Nelson in The Smurfs (Animated Series)

Iain Armitage

as Simon in The Smurfs (Animated Series)

Nat Faxon

as Weepy Smurf in The Smurfs (Animated Series)

Richard Steven Horvitz

as Mimic Smurf in The Smurfs (Animated Series)

Brian Tyree Henry

as Smooth Smurf in The Smurfs (Animated Series)

David Cross

as Social Smurf in The Smurfs (Animated Series)

Jimmy Fallon

as Passive Aggressive Smurf in The Smurfs (Animated Series)