Suggestions by @andymayer

Beau Weaver

as Mister Fantastic in Best Voices of Animated Characters

Bayonetta (Cereza)

as Anti-Heroes in Mount Rushmores

Asura (Asura's Wrath)

as Anti-Heroes in Mount Rushmores

Kratos

as Anti-Heroes in Mount Rushmores

Stocking Anarchy

as Anti-Heroes in Mount Rushmores

Panty Anarchy

as Anti-Heroes in Mount Rushmores

Ryuko Matoi

as Anti-Heroes in Mount Rushmores

Ghost Rider (Johnny Blaze)

as Anti-Heroes in Mount Rushmores

Hellboy

as Anti-Heroes in Mount Rushmores

Deadshot (Floyd Lawton)

as Anti-Heroes in Mount Rushmores

FAKE

as Anti-Heroes in Mount Rushmores

Tony Soprano

as Anti-Heroes in Mount Rushmores

E-123 Omega

as Anti-Heroes in Mount Rushmores

Rouge the Bat

as Anti-Heroes in Mount Rushmores

The Punisher (Frank Castle)

as Anti-Heroes in Mount Rushmores

Team Rocket

as Nintendo Villains in Mount Rushmores

Giygas

as Nintendo Villains in Mount Rushmores

Ridley (Metroid)

as Nintendo Villains in Mount Rushmores

Venom

as Anti-Heroes in Mount Rushmores

Wario

as Anti-Heroes in Mount Rushmores